Radon transport in permeable geological environments

Abstract

This article presents the results of a long-term soil radon and meteorological parameter monitoring study in the fault zone at Mt. Beshtau, North Caucasus, which for more than 3 years. Strong seasonal variations in the radon levels with maxima during summer and minima during winter were recorded. The values of radon exhalation and soil radon concentration have a range of 0.025–25 Bq m 2 s −1 and 1–170 kBq m −3, respectively. In addition, measurements of the air radon concentration, and direction of air movement at the adits mouths of the former uranium mine on the same mountain were carried out. Seasonal radon variations, similar to those observed in fault zones, were recorded at the mouths of adits. It was established that radon anomalies are associated with the periodic release of mine air from the fractures and tunnels into the atmosphere. Above an altitude of 900 m a. s. l., an abnormal release of radon occurs in winter, when the mine air is warmer than the surrounding atmosphere. At the altitudes below 900 m the cold radon rich air blows from the adit mouths in summer. During mine air discharge, radon concentrations in the open atmosphere locally around the adit mouth reach 600,000 Bq m−3, averaging 50,000–250,000 Bq m−3. The temporal pattern of radon fluctuations in fault zones and at the adit mouths is similar. A very close correlation between radon levels and atmospheric air temperature was observed both in the fault zone and at the adits mouths. It indicates that radon release in both cases are caused by a single mechanism. This mechanism probably is the atmospheric air circulation in shallow permeable zones due to the temperature difference between the inside mountain and ambient atmosphere.